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ORNL-TM-2571.txt
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«) ‘Q’\' 9
BN
)
«) ??
ORNL-TM-2571
Contract No. W-7405-eng-26
Reactor Division
THEORETICAT DYNAMIC ANALYSIS OF THE MSRE WITH 233U FUEL
Ro' c. Steffy, JI‘. .Pc Jo WOOd
- LEGAL IQC)TIC:E |
~ This report was prepared 28 an account of Government lponsored work, Nelther the Unltod
States, nor the Commission, nor any person acting ok behalf of the Commission:
A. Makes any warranty or representation, expre!aed or lmplied, with respect to the accu- |
i racy, completeness, or usefulness of the fnformation contained in this report, or that the use ;
! of any Information, apparatus, method, or process diaclosed in this report may not lntrlnga ;
privately owned rights; or !
t . ... B, Assumes any liabilities vlth respect to the n’e of, or for duna.gea resuitlng from the |
L. nse of any information, apparatus, method, or proceds disclosed in this report.
{ As used in the above, ‘‘person acting on beha of the Commission® fncludes any em-
! . ployee or contractor of the Commission, or employ of such contractor, to the extent that
.~ such employee or contractor of the Commission, o employee of such contractor prepares,
§ " diaseminates, or provides access to, any information pursuant to his employment or wntmct
i -with the Commuslon. or hl- employment with such contractor. . :
JULY 1969
OAK RIDGE NATIONAL LABORATORY
- Oak Ridge, Tennessee
operated by |
UNION CARBIDE CORPORATION
. for the .
U.S. ATOMIC ENERGY COMMISSION
GRIRIBUTION O gis COCUMENZ & UNTIMTED
t;_...fl
- _?‘
. &
e
)
&«) .
"
") Q» f
@?‘ o
iii
CONTENTS
“Abstract.........l......’C.’VO‘.Ol..'...""I.l.l...l.......‘......
-J-l IntrOduCtion QO..'.OO.-.l.O...'..l............f..O..'.O..O.I.'
2. Model Description and Verification ...cc.ecevcecccccceccnnesn
3, Transient-Response'Anglysis .......,.......;...,.............
4. Frequency-Response Analysis_.....;...........,.,............;
4.1 Calculated Frequehcy Response of Power bosReactivify .o
:4.1.1 For ancirculafiinglFuel..........................
4.1.2 For Circulating Fuel «.cecasenccrercccecacencnons
4.2 Effect bf'Mixing*in~the FUEl LOOD seesvocesasescsscnnsns
4.3 Sensitivity of 8n/ng-8k to:Parameter Changes ....eceee..
b4 Frequency'Responsé:of‘Outlet:Temperature-to=Powerr......
5. Stability Analysis .eececssscsccncscccnccnccrsresoccccconanes
5.1 Pole Configuration — Eigenvalues eeeeeececseccsansanncss
5.1.1 Theoretical DiscusSSiOnS ssccecscsccncenccnnccncne
5.1.2 Eigenvalue Calculation ReSUIES eeeececvececncesos
5.2 Modified MIKNAilov MethOR «eeeeseessenecsescassocnnsoens
5.2.1 Theoretical DiSCUSSION .eceeeevsscsccassacscosnns
5.2.2 -Results-of:Appiying"the Mikhailov Stability
,Criterion:o-_'-.-,....s-.-..-.r-.-..-.....-..........
6. CQHCludingDiscuSSion 8 8 8 8 O 0 0 8 5 T O 0 PSSO ET O PO NEESEPeSHSESEs s
‘ACkflOWledgnentS;...g.ob;..-..a.-.......-..-Q.......'...........-...
References ..............‘lOOQIVO;OO.UOIOCOIO.....-.'...C.Q..'.'......
Appendix. Pa,dé -Approximations.-.....;.C.‘...0...'.'........0'....
Page
o N H O
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A e
"
@) L
gk
THEORETICAL DYNAMIC ANALYSIS OF THE MSRE WITH 233U FUEL
R. C. Steffy, Jr. and P. J. Wood*
‘Abstract
A study undertaken to characterize the dynamics of the
233y.fueled MSRE prior to operation revealed that the system
is inHerently asymptotically stable at all power levels above
zero. The motivation for these studies was the expected dif-
ference between the MSRE dynamic response with 232U fuel and
‘with 23 U fuel because of the smaller delayed-neutron frac-
tion of 233y, An existing system model, previously verified
for 2357 fuel, was modified for use in this work. The reac-
tor system response_to reactivity perturbations is rapid and
nonoscillatory at high power, and it becomes sluggish and
oseillatory at lower powers. These characteristics were de-
termined by three methods: (1) transient-response analyses,
~including a check of the validity of the linear model, (2) a
frequency-response and sensitivity study, (3) stability analy-
ses, both by inspection of the system eigenvalues and by ap-
plication of the recently developed modified Mikhailov cri-
terion. .
Keywords: MSRE, 233U fuel, stablllty, elgenvalues,
modified Mikhailov crlterla, frequency response, sens1t1v1ty,
time response, Padé approximations.
1. Introduction
As a preliminary step in the development of a molten-salt-fueled
-breeder reactor, the Molten Salt Reactor Experiment (MSRE) was fueled with
_233U to perform the necessary physlcs and chemistry experlments on thls
:flrst 233U-fueled nuclear power reactor. Before nuclear operatlon, it was
1mportant to antlclpate the dynamlc behavior and the. 1nherent stability of
the system in order to insure safe, orderly operatlon and to plan safe,
,deflnltlve experlments.,
The principal motivation. for evaluatlng the operatlng characterlstlcs
of the 233U fueled MSRE after more than 70 000 Mwhr of power operatlon
wuth 235y fuel is that. 233y has & much smaller delayed-neutron fraction
*Currently- As31stant Dlrector of MIT School of Chemlcal Englneerlng
Practice at Oak Ridge National Laboratory.
2
~ (B) than that of 23°u. fhe.?33U'fue1 was expected to have operating char-
acteristics somewhet different from those of 233y and, in particular, a
faster response to feadtivity perturbations{ Table 1 lists the predicted
basic nuclear-kinetics properties of the MSRE with 233y fuel and compares
‘them with those of the reactor with %2°U fuel.
Several different technigues were used in analyzing the dynamiés of
the 23%U-fueled MSRE, primarily because .each technique either gave infor-
‘mation unavailable from the others or used different _approx:i.mate :fireat- _
ments to describe the system. In performing'the-dynamics analyses a model
developed by Ball and Kerlin' was modified slightly and used to -describe
the MSRE with ?32U fuel. (This model did not include the effect of ‘the
réaétor control system.) The tifie'response of the reactorfsystem to a
reactivity perturbatlon at several power levels was calculated first. The
‘computer code.NmEEXP which calculates the time response of a multivari-
able nonlinear system with pure time delays, was used in this study. Next
~the syStem frequency response was determined by using the computér code
'SFR-3 (Ref. 3). This code was also used to .determine amplitude ratio (or
‘gain) sensitivity'to‘changes in the system variables (i.e., the ratio.of
‘the change in amplitude ratio to the correspbnding change-inra'éystem_varif
-able was determined as a function of‘fréquency). Finally, the absolute
stability of the system was investigated by two techniques. The_system
eigenvalues were calculated at several powers to determine whether oscil-
latiqns.in&uced in the system would increase or decrease in amplitude,
and the Mikhailov stability criterion, as modified by Wright ‘and Kerlin,*
wag used to obtain this same information with fewer approxnmatlons in the
mathematlcal model.
Linearized system equations were- used in the frequency-response and
sensitivity calculations and in both types of stability analysis. This
was-ngcessary'because-general calculational methods do not presently exist
.that would permit ‘these types of analysis'with 8 set of nonlinear system
‘equations. The;time-response calculations utilized the nonlinear equa~
tions. This was possible because they involved an iterative procegdure
that provided for -updating the nonlinear terms after each itefation.
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Table 1. Comparison of Nuclear Parameters Used in Dynamics Analyses
of MSRE with 273U Fuel and with 235U Fuel
233y Fuel
23 5U Fuela
‘Bi,=Delayed~Néutron.
Group Ay Deéay | Fraction
Aj, Decay
By, D61ayed—NEutron
Fraction
C?nsta?§ . — C?nstagg —
sec” i Circulating, (sec” s Circulating,
| - Steble Chprective | Static rrective
- | X 1074 x 1074 . X 10™% X 10™4
1 . 0.0126 2,28 11,091 0.0124 -2.23 - 0.52
2 - 0.0337 = 7.88 3.848 0.0305 - 14.57 3,73
3 0.139 . 6,64 4.036 0.111 - 13.07 4,99
4 0.325 - 7.36 5,962 0. 301 26. 28 16.98
5 1.13 : 1.36 1.330 1.14 7.66 7.18
6 2.50 0.88 0.876 3.01 2.80 2.77
Total B 26.40 17.14 Total B 66.61 36.17
Prompt neutron generation 4 X 10~% 2.4 x 1074
time, sec : ,
Temperature coefficients
of reactivity, °F | -
Fuel salt - —6,13 X 10°° —4.84 X 1075
Graphite | -3.23 x 1077 -3,70 x 10>
&Dats from Ref. 1.
”
4
2. Model Description and Verification
A mgthematical model was reguired-to:describe the dynamic behavior
of the ???U-fueled MSRE. The model chosen for ‘this study was essentially
that called the "complete model" in Ref. 1, which was developed to analyze
the dynamics of the 235y. fueled MBRE. The'justification for using this
model was its good agreement with experlmental results when applled to
the 23°y-fueled system.’ -
Some changes were made in the model of Ref. 1, howéver, before it
was applied to the *32U-fueled system. The experimental results of the
previous testing program did not verify the dip in the calculated frequency
response cfirve at approximately 0.25 radian/sec, .which. corresponds to a
fuel circulation time of approximately 25 sec. This was attributed to .in-
sufficient'mixing of fuel salt in the .external loop of the .theoretical
model. To provide the model with more mixing, an additiopai 2-sec first-
order time lag (mixing pot) was incorporated at the core outlet. This is
a reasonsble approximation for the mixing in the upper and lower reactor-
vessel plenums. - ;
The chief features of the 44th-order model shown in Fig. 1, are the
fbllow1ng.
B 1. The reactor core was divided into nine regions, each of which
was split into two fuel lumps and one graphite lump. Consideration was
given to the nuclear importance of thermal disturbances in each of the
lumps. (The term "lump" as used in mathematical modeling refers to a seg-
ment'of a physical system that is considered.to have constant\prdperties
throughout and which interacts with its surroundings through only those
properties. ) : |
‘2. A five-lump representatipn of the fuel-to-coolant heat exchanger
was used, with heat being exchanged to a single metal lump at the tempera-
ture of the fuel leaving the first of two fuel lumps and heat being ex-
-changed from the metal lump to the coolant at:fhe‘outlet;temperature of
“the flrst of two coolant lumps.
3, A three-lump coolant-to-air radiator. was used in which the coolant
-transferred heat to a single metal lump at the temperature of the coolant
leaving the first of two coolant lumps.
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ORNL-DWG 68—10067R
3.77-sec DELAY
1
1 4.74sec DELAY
l
2-sec MIXING POT | '
| : ] AIR
‘ 4 7 9 - ' - , STREAM
FUEL COOLANT COOLANT 3
LUMP LUMP LUMP
3 6 §
MSRE GCORE
(9 REGIONS) ,
8 - --| METAL }--+ -~ = [METAL} --1
FUEL GOOLANT COOLANT
. LUMP LUMP LUMP
i } ] ] ‘ - i
FUEL-SALT HEAT 1 rebiaton
|
| | EXCHANGER 8.24-sec DELAY
8.67-sec DELLAY
Fig. 1. Schemeatic Drawing of MSRE Showing System Divisions Used in
Mathematical Analysis. = .
%
4. A linear model of the reactor kinetics equations was used in all
studies, except the time-response calculations,‘in.which.nonlinear'kinetics
effects were taken into account. . |
5. The neutron kinetics equatiohs were represented by a mathematical
~expression that accounted for the dynamic effect of circulating precursors
(except for the eigenvalue calculatlon, which required the use of effec-
tive delayed-neutron fractlons)
6. Xenon poisoning was assumed to be at steady state and not influ-
‘enced by small perturbations.
3. Transient-Respbnse Analysis
Time responses were obtained at several power levels to provide a -
-physical picture of the reactor response to réactivity perturbations such
as control rod motions. The computer code MATEXP? applied in this analy-
sis makes use of the matrix exponentiation technique of solving a.syStem'
of nonlinear ordinary differential equations (with pure time delays) of
the form | |
= Ax + MA(x) x + £(t) , (1)
?f-|§‘|
where
x = the solution vector (system state variables), =
A = system matrix (constant square metrix with real coefficients),
AM(X) = a matrix whose elements are deviations from the values in A,
[thus AA(%) x includes ‘a1l nonlinear effects and time delay
terms],
f(t) = foreing function.
The predicted response of the reactor power to a step reactivity in-
erease of 0.02% 8k/k is shown in Fig., 2 for various initial powers. These
response curves point out several important characteristics of the MSRE.
At 8 Mw the maximum power level is reached during the first second after
-tfie step reactivity input. The rapid increase in reactor power is accom-
-panied by a rapid increase in fuel température in the coré, which, coupled
with the negative temperature coefficient of reactivity, more than
¥)
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"
& POWER (Mw)
A POWER (Mw)
13 ORNL-DWG 68-{0077R
1.0
o8
0.6
04
A PONER {(Mw)
02
-0.2
08
0.6
0.4
0.2
~0.2 |
A POWER (Mw)
A POWER (Mw)
~04
-0.20
0.16
042
0.08
0.04
-0.04
-0.08 -
O 100 200 300 400 500 £00 TOO 800 ! 800 - 1000
B ' “TIME (sec) ' '
' Fig. 2. Calculated Power Response of the 233U-Fueled MSRE to a
- 0.02% Bk/k Step Reactivity Insertion at Various Power Levels.
8
counterbalances the step reactivity input, so the power lével_begins'to . kfi’
decrease. The temperature of the salt entering the core is constant -dur- |
‘ing this interval, and when the power has decreased enough for the reac- *
-‘tivity associated with the increased nuclear average temperature to just
cancel the step reactivity input, the power levels for a brief time (from
~6 to ~17 sec after the reactivity input). About 17 sec after the reac-
tivity increase, the hot fluid generated in the ihitial'power\increase
has completed its circuit of the loop external to the core, and the nega-
tive temperature coefficient of the salt again reduces the reactivity so
that the power level starts down again. At large times the reactor power
‘has returned to its initial level, and the step reactivity input has been
-:counterbalanced»by an increase in the nuclear average temperature in the
core. The short plateau observed in the time-response .curve at.8 My was
also noted in the 5-Mw case. - At lower powers, however, the élower system
response-prevents the reactor from reaching the peak of its first oscilla-
tion before the fuel has completed one circuit of the external fuel loop.
The plateau therefore does not appear in the lower pdwer cases.
-An important characteristic of the MSRE dynamic response is that as
-the power is decreased the reactor becomes both sluggish .(slower respond-
)
~ ing) and oscillatory; that is, at low powers the time required for oscil-
lations to die out is much larger than at higher powers, and the fractional
amplitude of the oscillations (A‘power/power) is larger.
As part of the time-response analysis, the validity of the linear ap-
proximation for reactivity perturbations roughly equivalent:to 1/2.in. of
‘control rod movement (0.04% 8k/k) was checked. The results of this analy-
sis are shown in Figs. 3 and 4 for 8- and 0.1-Mw operation. At 8 Mw the
linear approximation is fairly good, but at 0.1 Mw it is;pocr. This re-
sult can be understood by considering the general form of the neutron-
kinetics equations:
ddn pg ~ Br ng 5p & Spdn
— e &n + -+ A0, + =, = ’
dt l z i=1 I
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u B ORNL —DWG 68—10065R
' 2.5
* | ' — 2.0\
'\ ' ——NONLINEAR
.| —=——LINEAR
]
|
A POWER (Mw)
»
-
(7
1.0 _
\
N -
0.5 \\
. BE \'
0
0 BRI [+ ] 20 30 40 50
TIME(sec)
Fig. 3. Power Response of the 233U-Fueled MSRE Ini’cially Opereting
~at 8 Mw to a 0.04% Step Reactivity Insertion as Calculated with anlinear
and Iinearized Kinetics Equations.
n
~ ORNL—DWG 68—{00€6R
]
0.5 : NONLINEAR /
| | =——LinEAR /
0.4 ' /
/
0.2 _ ' |
A POWER {(Mw)
o
w
\\
1=
|
0 —L |
__ 0 10 20 30 40 50
'_' ' TIME (sec) '
% | SR Fig. 4. Power Response of the 233y-Fueled MSRE Initially Operating
at 0.1 Mw to a Step Reactivity Insertion of 0.04% as Calculated m.th
g Nonlinear and Linearized Kinetics Equations.
10
where
on = deviation of power from its initial value (ng),
po = reactivity necessary to overcome effect of'fuel circulation,
fiT = total delayed-neutron fraction,
! = neutron generation time in system,
Op = deviation of reactivity from its initial value,
A\; = decay constant for ith delayed-neutron precursor,
Sci = concentration of ith delayed-neutron precursor.
The last term in Eq. (2), 5p8n/I, is the nonlinear term. In the
8-Mw case the maximum deviation of the power from the initial power is
only about 30% of the initial power, whereas in the 0.1-Mw case the maxi-
mum deviation is 560% of the initial power and is still increasing after
50 sec. When the dn term is this iarge-with respect to:the'no'term, the
nonlinear terms in the kinetics equation play a much larger fole.than-the
linear terms. Thus, neglecting the nonlinear terms may lead to signifi-
cant ‘error if the power -deviates from its initial level by more than a
few percent. For the time-response analysis, it was neceséary'to include
the nonlinear terms to obtain realistic resfilts; however, use of the lin-
earized equations in the frequency-domain analysis (Section 4 of this re-
port) is acceptable because the analysis is based on small reactivity and
power perturbations that oscillate around their initial values.
4. Frequency-Response Analysis
Because ‘a closed-loop frequency-response analysis provides informa-
tion about relative system behavior, the linear MSRE model was studied at
different power levels from this point of view. The linear system equa-
tions were first Laplace transformed and then solved for the ratio of an
output variable (such as power or temperature) to an input varisble (such
as reactivity). This ratio, called a transfer function, is
¥)
”
0
n
11
where
G(S) = transfer function,
0(S) = the output variable,
I(S) = input variable,
S = Laplace.transformeariable.
For & stable system, S may be replaced by jw, where J = V-1 and w is the
ifrequency of an input sine wave. With this substitution, G(jw) is a com-
plex number; the magnitude of G(jw) is called the gain or the magnitude
ratio and is the ratio of ‘the amplitude of an input sinusoid to that of
an output sinusoid. The phase of G{jw) is the phase difference between
the input and the output sinusoids. A plot of G(jw) and the phase of
G(Jw) versus .w is referred to as a Bode diagram or a frequency-response
plot. A Bode plot provides qualitative stability information in the peaks -
of the magnitude ratio curves. - High, narrow peaks indicate lower stability.
“than flatter, broader peaks.
There are two basic reasons for calculating the frequency response
of a system. First, the frequency-response curves are good 1ndlcators-of
system performance, and seeohd,:the frequency response of a system may be
~experimentally determined. The latter consideration is important because
it provides a means for checking the validity of a model. - When the ex-
- perimentally determined frequency response of the system is in agreement
with that of the theoretical model, confidence is gained in the conclusions
‘drawn from the stability analysis applied to the model.
4.1 Calculated Frequency'ReepenSe of Power to Reactivity
4;1.1 .For aneirculatifinguel.' The calculated'frequeney‘response
-of the MSRE for‘the‘noncirculating,~zero-power,.233Uqueled condition is
, shown in- F1g.-5. These . curves are very 31milar t0 those of the c15881c
zero-power reactor, and reference curves may be found in most textbooks
" on reactor dynamics.®57 AtfzerOTpower, temperature feedback effects are
not ‘important, so.the calculated response is that of ‘the neutron-kinetics
‘equations.
4.1.2 For Circulating'Fuel; A.setiof'frequency—response'curvesvfor
“circulating 223U fuel is shown in Fig. 6. These curves show the effect
40,000
12
ORNL—DWG 68 — {00T9R1